To add the PPA, run the following terminal commands:
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sudo add-apt-repository ppa:libreoffice/libreoffice-4-0
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sudo apt-get update
Adding the main LibreOffice PPA which will get updates not only with LibreOffice 4.0.x but also newer versions, use the following commands:
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sudo add-apt-repository ppa:libreoffice/ppa
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sudo apt-get update